CHAPTER 14 (cont.), LECTURE 2:

New example:  Given:  A + B + C ----> Prods.
    Find the rate law and k (specific rate constant).

                          [A]       [B]       [C]      initial rate (Ms-1)
          exp.1      0.20      0.10    0.90     1.8 x 10-2
          exp.2      0.10      0.20    0.30     3.0 x 10-3
          exp.3      0.20      0.20    0.30     1.2 x 10-2
          exp.4      0.20      0.20    0.10     4.0 x 10-3
 

                rate = k[A]x[B]y[C]z

1)   Compare exps. 4 & 3:
rate 4 =4.0 x 10-3  = k[A]x[B]y [C]z=k(0.20)x(0.20)y(0.10)z
rate 3    1.2 x 10-2     k[A]x[B]y [C]z     k(0.20)x(0.20)y(0.30)z

     4.0 x 10-3 = 4.0  = 0.333 = (0.10)z = (0.333)z
   1.2 x 10-2    12.0                   (0.30)z

                Therefore, z = 1
 

2)   Compare exps. 2 & 3:
rate 3 =1.2 x 10-2  =k[A]x[B]y [C]z=k(0.20)x(0.20)Y(0.30)z
rate 2    3.0 x 10-3    k[A]x[B]y [C]k(0.10)x(0.20)Y(0.30)z

   1.2 x 10-2= 12.0 = 4.0 = (0.20)x = 2x        Therefore, x = 2
     3.0 x 10-3      3.0                      (0.10)x
 

3)   Compare exps. 1 & 3:
rate 1 =1.8 x 10-2  =k[A]x[B]y [C]z=k(0.20)x(0.10)Y(0.90)z
rate 3    3.0 x 10-3    k[A]x[B]y [C]z   k(0.20)x(0.20)Y(0.30)z

1.8 x 10-2 = 1.8 = 1.5 = (0.10)y(0.90)z
1.2 x 10-2     1.2                    (0.20)y(0.30)z

                   =(0.5)y(3)z =(0.5)y(3)1

                              1.5 = (0.5)y(3)

              1.5 = (0.5)y;   0.5 = (0.5)y            Therefore, y = 1
               3

We now have the values for x, y , z, and therefore have
        the rate law

                rate = k[A]x[B]y[C]z  = k[A]2[B]1[C]1
 

We can now calculate k, the specific rate constant:
 1.8 x 10-2 Ms-1 = k(0.20M)2(0.10M)1(0.90M)1

        k =        1.8 x 10-2Ms-1              = 5.0 M-3s-1
              (0.20M)2(0.10M)(0.90M)
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14.3 Relation Between Reactant Concentration and Time
Concentration vs. Time:  Integrated rate equation

We can use this to find out how much of a reactant remains
after a specified amount of time.  We can also find out what
the half-life, t1/2, the time it takes for 1/2 of that reactant
to be used up.  These are different for different orders of
reactions.  We will be looking at only one reactant going to
product.

0th-Order Reactions:    for me:  check this all out!!!!!!!!!

    aA -----> Products:  if the reaction is 0th order in A
                                       and 0th order overall, then:

              Rate = k[A]0 = k = -(1/a)(D[A]/Dt)

    which means that the rate is independent of the
    concentration of A.

The integrated equation is:  [A] = [A]o - akt

And the half-life is:   t1/2 = [A]o/2ak  (THIS IS ONLY
                                                            FOR 0th ORDER!!)

Therefore, a linear plot of [A] vs. time yields a straight
     line function, where y = mx + b, and
     m = slope = -k  and b = the y-intercept at time 0

UNITS of k are:  Mtime-1  =  Ms-1  = Mmin-1  = Mhr-1
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1st-Order Reactions:

    aA -----> Products:  if the reaction is 1st order in A
                                       and 1st order overall, then:

                            Rate = k[A]1

which means that the rate is directly dependent on the
                concentration of A.

The integrated equation is:     ln([A]/[A]o) = -akt

        where:  [A]= initial concentration of A
                      [A]   = concentration of A at some time t
                         a    = coefficient in the balanced equation
                         k    = specific rate constant
                         t    = time after reaction begins

And the half-life is:   t1/2 = 0.693/ak   (THIS IS ONLY
                                                                FOR 1ST-ORDER!!)

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Derivation of 1st order integrated rate equation:

rate = -D[A]/aDt = k[A]1

            (D[A])/[A]  = - akDt

Integrate left-hand side from Ao to A and the right side
                from t = 0 to t = t:

             ln([A]/[Ao]) = - akt

            ln[A] - ln[Ao] = - akt
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Therefore, a linear plot of [A] vs. time yields an exponential
    decaying curve; a plot  of ln[A] vs. time yields a straight
    line function, where y = mx + b, and
         m = slope = -ak      and
          b = the y-intercept at time 0 = ln [A]o

UNITS of k are:   Rate = k[A]
                       
Rate/[A]1 = k  ; therefore, Ms-1/M = time-1
 

Ex.:  The decomposition of N2O5 to NO2 and O2 is 1st order,
    with a rate constant of 4.80 x 10-4/s at 45oC.  If the initial
    concentration of N2O5 is 1.65 x 10-2 mol/L, what is the
    concentration after 825 s?

Balance the equation!!!   2 N2O5(g) ----> 4 NO2(g) + O2(g)

                 ln([A]o/[A]) = akt
            ln[A]o- ln[A] = akt
     ln (1.65 x 10-2M) - ln[A] = akt = 2(4.80 x 10-4/s)(825s)
            -4.104 - ln[A] = 0.792
                        - ln[A] = 0.792 + 4.104 = 4.896
                           ln[A] = -4.896
                              [A] = 0.00747 M = 7.47 x 10-3 M

How long would it take for the concentration of N2O5 to
    decrease to 0.950 x 10-2 mol/L from the initial value
    given above?

           ln([A]o/[A]) = akt
       ln (1.65 x 10-2 M/0.950 x 10-2 M) = 2(4.80 x 10-4/s)(t)
       ln(1.737) = (9.60 x 10-4/s)(t)
       0.552/(9.60 x 10-4/s) = t
                                   575 s = t
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DERIVATION OF 1/2-LIFE:

         ln([A]o/[A]) = akt

          ln([A]o/([A]o/2)) = akt1/2

       ln(1/2) = akt1/2

       ln2 = akt1/2

       0.693 = akt1/2
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At 25oC, the specific rate constant for a reaction A ---> B
    is 0.0450 s-1.....Therefore, 1st order!!  What is the
    half-life of A?

     t1/2 = 0.693/ak
      t1/2  = 0.693/1(0.0450 s-1) = 15.4 s
  This means that 1/2 of A is gone after 15.4 s, another 1/2
    of the 1/2 is gone after another 15.4 s (therefore only
    1/4 is left!!), etc.

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2nd Order Reactions:

    aA -----> Products:  if the reaction is 2nd order in A
                                       and 2nd order overall, then:

                            Rate = k[A]2

The integrated equation is:   (1/[A]) - (1/[A]o) = akt

        where:  [A]= initial concentration of A
                      [A]   = concentration of A at some time t
                         a    = coefficient in the balanced equation
                         k    = specific rate constant
                         t    = time after reaction begins

And the half-life is: t1/2 = 1/ak[A]o    (THIS IS ONLY
                                                             FOR 2nd ORDER!!)

Therefore, a linear plot of [A] vs. time yields an exponential
    decaying curve; a plot  of ln[A] vs. time also yields an
    exponential decaying curve; a plot of 1/[A] vs. time
    yields a straight line function, where y = mx + b,
    and m = slope = ak  and
            b = the y-intercept at time 0 = 1/[A]o

UNITS of k are:  Rate = k[A]2
                           
Rate/[A]2 = k; therefore, Ms-1/M2 = M-1time-1
 
 

Real-Life Example:  Decomposition of NO2
                        2NO2(g)  ---->  2NO(g) + O2(g)

        Time(s)        [NO2]        ln[NO2]        1/[NO2]
              0             0.0100        -4.60             100
            60             0.0068        -4.99             147
          120             0.0052        -5.26             192
          180             0.0042        -5.47             238
          240             0.0035        -5.65             286
          300             0.0030        -5.81             333
          360             0.0026        -5.94             385

1)  Plot [NO2] vs. time and get an exponential decay;
        therefore, NOT 0th order !!!
2)  Plot ln[NO2] vs. time and get another exponential
        decay; therefore, NOT 1st order !!!
3)  Plot 1/[NO2] vs. time and get a straight line;
        therefore, the reaction IS 2nd order !!

      slope = ak = Dy/Dx = (333-100)/(300-0) = 0.777
      therefore, k = slope/a = 0.777/2 = 0.388
M-1s-1

and t1/2=1/ak[A]o=1/[2(0.388M-1s-1)(0.0100M)]=129 s

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