CHAPTER 21- NUCLEAR CHEMISTRY - Lecture 1:

Radioactivity : Alpha-, beta-, and gamma-Rays

The three main types of radiation are:-
1.  large mass, positively charged radiation (alpha a),
            high speed helium nuclei, 42a, 42He, +2
            charged particle.
2. small mass, negatively charged radiation (beta b) ,
            high speed electrons, 0-1b, 0-1e, -1 charged
            particle.
3. high energy electromagnetic radiation (gamma g),
            loss of a high energy photon from the nucleus,
            no charge.

The relative penetrating power: a = 1; b = 100; g = 10000.
 

Radioactivity:

Some heavy elements spontaneously emit radiation =
    called radioactive.
 23392U   23592U     23892U  are all radioisotopes of Uranium
All of these have 92 protons and 92 electrons, and either 141,
     or 143, or 146 neutrons, respectively.

They also  have different % natural abundances:

U238  is 99.3%; U235 is 0.7% and U233 is trace.
 

Henri Becquerel worked with K2UO2(SO4)2.  Put it on film
    and it blackened it.
Pierre and Marie Curie isolated Po and Ra from pitchblende.
     They received the Nobel prize for this work in 1903.
 

Nuclear Equations:
     Nucleons: particles in the nucleus:
             p+: proton
             n0: neutron.
 Mass number: the number of p+ + n0.
 Atomic number: the number of p+, also = number of electrons
 Isotopes: have the same number of p+ and different
            numbers of n0

In nuclear equations, the total number of nucleons is
    conserved:

  23892U -----> 23490Th  + 42He    radioactive decay
  13153I  -----> 13154Xe + 0-1e

  9943Tc  -----> X + 0-1e    Find X.      9944X, therefore X = Ru
 

 In the decay of 131I, an electron is emitted.  For balancing
    purposes, we assign the electron an atomic number of -1.
 The total number of nucleons before a nuclear reaction
    must be the SAME as the total number of nucleons after
    the reaction.
 

Types of Radioactive Decay:
 In nuclear chemistry, to ensure conservation of nucleons,
    we write all particles with their atomic and mass numbers:
    42He and 42a both represent alpha-radiation.

 Nucleons can undergo decay:
  10n -----> 11p  + 0-1e    (beta-emission)
  01e + 0-1e  ----->      (positron annihilation)
  11p -----> 10n  + 01e     (positron or beta+emission)
  11p + 0-1e -----> 10n     (electron capture)

 A positron is a particle with the same mass as an electron
    but with a positive charge.

Patterns of Nuclear Stability:

All nuclei with 83 or more protons are radioactive.

Neutron-to-Proton Ratio
 The proton has high mass and high charge.
 Therefore the proton-proton repulsion is large.
 In the nucleus, the protons are very close to each other.
 The cohesive forces in the nucleus are called strong
        nuclear forces.  Neutrons are involved with the strong
        nuclear force.
 As more protons are added (the nucleus gets heavier),
        the proton-proton repulsion gets larger. Therefore, the
        heavier the nucleus, the more neutrons are required for
        stability.
 The belt of stability deviates from a 1:1 neutron to proton
        ratio for high atomic mass.
 At Bi (83 protons), the belt of stability ends and all nuclei
        are unstable.

1. Nuclei above the belt of stability undergo beta- emission.
        An 0-1e (beta) is ejected from the nucleus when a neutron
        is converted into a proton.   10n -----> 11p  + 0-1e
2. Nuclei below the belt of stability undergo positron emission
        or electron capture.  Positrons are emitted when protons
        are converted to neutrons.     11p -----> 10n  + 0+1e
3. Nuclei with atomic numbers greater than 83 usually
        undergo alpha-emission.
 

Radioactive Disintegration Series:
 A nucleus usually undergoes more than one transition on its
        path to stability.
 The series of nuclear reactions accompanying this path is
        the radioactive series.
 Nuclei resulting from radioactive decay are called daughter
        nuclei.
 For U-238, the first decay is to Th-234 (alpha-decay).
    The Th-234 undergoes beta- emission to Pa-234 and U-234.
    U-234 undergoes alpha-decay (several times) to Th-230,
    Ra-226, Rn-222, Po-218, and Pb-214.  Pb-214 undergoes
    beta- emission (twice) via Bi-214 to Po-214, which
    undergoes alpha-decay to Pb-210.  The Pb-210 undergoes
    beta- emission to Bi-210 and Po-210, which decays (alpha)
    to the stable Pb-206.

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